$Rev:: 561 $ $Date:: 2011-12-13#$ 1 0 0 0 9.524100+4 2.389860+2 1 1 0 49543 1451 1 0.000000+0 0.000000+0 0 0 0 69543 1451 2 1.000000+0 3.000000+7 1 0 10 79543 1451 3 0.000000+0 0.000000+0 0 0 449 1269543 1451 4 95-Am-241 LANL EVAL-Oct10 T.Kawano,M.B.Chadwick 9543 1451 5 DIST- 20111222 9543 1451 6 ----ENDF/B-VII.1 MATERIAL 9543 9543 1451 7 -----INCIDENT NEUTRON DATA 9543 1451 8 ------ENDF-6 FORMAT 9543 1451 9 9543 1451 10 **************************************************************** 9543 1451 11 Modification to ENDF/B-VII.0 9543 1451 12 T. Kawano, M.B. Chadwick, A. Kahler, P.G. Young 9543 1451 13 [Oct. 2010, Aug. 2011] 9543 1451 14 9543 1451 15 MF=2 Resonance Parameters 9543 1451 16 ENDF/B-VII.0 resonance parameters (were from ENDF/B-VI) 9543 1451 17 were replaced by the JENDL-4 resonance parameters. 9543 1451 18 The energies of resolved resonances are almost identical 9543 1451 19 to the values in ENDF/B-VI, but spins and widths show 9543 1451 20 some differences. 9543 1451 21 9543 1451 22 In the unresolved resonance range, we adopted LSSF=1, 9543 1451 23 so that the dilute cross sections are now given in File 3. 9543 1451 24 9543 1451 25 MF=3 Neutron Cross Sections 9543 1451 26 MT=18 9543 1451 27 We performed a SOK analysis in the entire energy range to 9543 1451 28 obtain both the cross sections and its covariance. 9543 1451 29 The energy boundary was lowered to 150 eV. The subthreshold 9543 1451 30 cross sections are now given in File 3. 9543 1451 31 MT=102 9543 1451 32 The capture cross section was re-evaluated with the 9543 1451 33 Hauser-Feshbach calculations (CoH3), which reproduces 9543 1451 34 the DANCE experimental data and an integral measuremnt. 9543 1451 35 9543 1451 36 MF=32 Resonance Parameter Covariance 9543 1451 37 Take from JENDL-4, as for the resonance parameters. 9543 1451 38 9543 1451 39 MF=33 Neutron Cross Section Covariances 9543 1451 40 The covariance matrices for the total, inelastic, (n,2n), 9543 1451 41 (n,3n), (n,4n), and capture cross sections were calculated 9543 1451 42 with KALMAN, combining the statistical model calculations 9543 1451 43 with available experimental data. 9543 1451 44 The covariance matrix for the fission cross section was 9543 1451 45 obtained with the SOK code. 9543 1451 46 9543 1451 47 9543 1451 48 **************************************************************** 9543 1451 49 9543 1451 50 P.Young [10/26/06] 9543 1451 51 Modified MF=13,MT=3 continuum x/s following the prescription by 9543 1451 52 H.Trellue and R.Little to correct problems in running MCNPX. Also 9543 1451 53 regridded MF=13,MT=3 summed x/s, added MF=15,MT=3 dummy spectrum 9543 1451 54 at 1.e-5 eV, and corrected gridding problems & inconsistencies 9543 1451 55 between MF=3 and MF=9. 9543 1451 56 9543 1451 57 **************************************************************** 9543 1451 58 Modification to ENDF/B-VI Rev. 2 9543 1451 59 9543 1451 60 MF=3 Neutron Cross Sections 9543 1451 61 MT=2 9543 1451 62 Adjusted to that cross sections sum to total. 9543 1451 63 MT=16,17 9543 1451 64 GNASH calclautions, and the parameters were adjusted to 9543 1451 65 reproduce the experiemtal data of Lougheed [Lo01], 9543 1451 66 Filatenkov [Fi99], and LANL C-INC data. 9543 1451 67 MT=18 9543 1451 68 The SOK code was used for evaluating the fission cross 9543 1451 69 section from 6 to 17 MeV. GNASH calculation was adopted 9543 1451 70 at high energies. 9543 1451 71 MT=102 9543 1451 72 Hauser-Feshbach statistical model calculations, and 9543 1451 73 renormalized to the experimental data of Gayther [Ga77], 9543 1451 74 and Wisshak [Wi80]. 9543 1451 75 MF=9 Multiplicities for production of radioactive elements 9543 1451 76 MT=102 9543 1451 77 Re-evaluated based on the GNASH calculation and 9543 1451 78 experimental data of Shinohara [Si97], and LANL C-INC. 9543 1451 79 9543 1451 80 Fi99 A.A. Filatenkov, RI-252, Khlopin Radium Institute (1999). 9543 1451 81 9543 1451 82 Ga77 D.B. Gayther, B.W. Thomas, Proc. 4th All Union Conf. 9543 1451 83 on Neutron Physics, Kiev, 1977, Vol.3, p.3 (1977). 9543 1451 84 9543 1451 85 Lo01 R.W. Lougheed, et al., UCRL-ID-145592, LLNL (2001). 9543 1451 86 9543 1451 87 Si97 N. Shinohara, et al., J. Nucl. Sci. Technol., 34, 7 (1997). 9543 1451 88 9543 1451 89 Wi80 K. Wisshak, F. Kaeppeler, Nucl. Sci. Eng., 76, 148 (1980). 9543 1451 90 9543 1451 91 **************************************************************** 9543 1451 92 EVALUATION OF n + 241Am REACTIONS 9543 1451 93 9543 1451 94 P. G. Young and D. G. Madland 9543 1451 95 9543 1451 96 Theoretical Division 9543 1451 97 Los Alamos National Laboratory 9543 1451 98 Los Alamos, NM 87545 9543 1451 99 February 23, 1994 9543 1451 100 9543 1451 101 I. SUMMARY 9543 1451 102 9543 1451 103 The cross section data file for neutron reactions with 241Am 9543 1451 104 has been reevaluated over the incident neutron energy range from 9543 1451 105 0.01 to 30 MeV. The evaluation is in ENDF-6 format. Details of 9543 1451 106 the analysis are given in the sections that follow. Some 9543 1451 107 general features of the work are: 9543 1451 108 9543 1451 109 1. The ENDF/B-VI n + 241Am resonance parameters were adopted at 9543 1451 110 neutron energies below 30 keV, suitably joined with the results 9543 1451 111 of the present analysis at 30 keV. 9543 1451 112 9543 1451 113 2. A coupled-channel optical model potential was developed from 9543 1451 114 analyses of nearby actinides that is consistent with 9543 1451 115 measurements of the n + 241Am neutron total cross section. This 9543 1451 116 potential was used to calculate the neutron total cross section, 9543 1451 117 elastic and inelastic scattering cross sections and angular 9543 1451 118 distributions, and reaction cross sections and transmission 9543 1451 119 coefficients for a theoretical analysis of the reaction 9543 1451 120 channels. The direct cross sections from the coupled-channel 9543 1451 121 analysis were combined with compound nucleus calculations at 9543 1451 122 lower energies and with preequilibrium theory calculations at 9543 1451 123 higher energies. Angular distributions for the first 40 excited 9543 1451 124 states of 241Am were obtained from the direct, compound-nucleus, 9543 1451 125 and preequilibrium calculations, and energy-angle correlated 9543 1451 126 distributions are provided for all continuum neutrons. 9543 1451 127 9543 1451 128 3. The evaluated fission and total cross sections were obtained 9543 1451 129 by adjusting the theoretical cross sections as needed to match 9543 1451 130 the available experimental data. 9543 1451 131 9543 1451 132 4. Nubar and the fission neutron spectra were obtained using 9543 1451 133 Madland-Nix theory. 9543 1451 134 9543 1451 135 II. THEORETICAL ANALYSIS 9543 1451 136 9543 1451 137 The primary goal of the theoretical analysis was to provide a 9543 1451 138 consistent set of data for all reactions over the energy range 9543 1451 139 30 keV to 30 MeV. In the case of n+241Am, there are reasonable 9543 1451 140 experimental data available for the neutron total and fission 9543 1451 141 cross sections. Therefore, the function of the theoretical 9543 1451 142 analysis was to provide the elastic, inelastic, (n,2n), (n,3n) 9543 1451 143 and (n,4n) cross sections, as well as the angular and energy 9543 1451 144 distributions of secondary neutrons. To accomplish this, a 9543 1451 145 theoretical analysis was performed, adjusting the relevant 9543 1451 146 parameters to match the total, fission, and (n,g) cross 9543 1451 147 sections. Additionally, a theoretical analysis was performed to 9543 1451 148 obtain the average neutron multiplicity from fission and the 9543 1451 149 energy spectra of fission neutrons as a function of incident 9543 1451 150 energy. 9543 1451 151 9543 1451 152 Coupled-channel deformed optical model calculations were 9543 1451 153 performed with the ECIS code (Ra70) over the incident neutron 9543 1451 154 energy range from 0.001 to 30 MeV. Hauser-Feshbach reaction 9543 1451 155 theory calculations were carried out with the LANL version of 9543 1451 156 the COMNUC code (Du70) at lower energies and the GNASH 9543 1451 157 statistical/preequilibrium code (Yo92) at higher energies to 9543 1451 158 obtain all partial reaction cross section data. Both reaction 9543 1451 159 theory codes used neutron transmission coefficients from the 9543 1451 160 optical model analysis. 9543 1451 161 9543 1451 162 A. Optical Model 9543 1451 163 9543 1451 164 The optical model potential was obtained by considering 9543 1451 165 several coupled-channel parameterizations developed from n + 9543 1451 166 235,238U and 239Pu experimental data (Ma78, Yo88, Yo92a). 9543 1451 167 Parameters were adjusted until a reasonable fit to experimental 9543 1451 168 data for the neutron total cross section of 241Am was obtained. 9543 1451 169 The lowest five members of the 5/2- ground state rotational band 9543 1451 170 were included in the calculations, that is, the 7/2-, 9/2-, 9543 1451 171 11/2- and 13/2- excited states at Ex = 41, 94, 159 and 235 keV 9543 1451 172 were coupled with the 5/2- ground state. 9543 1451 173 9543 1451 174 B. Reaction Theory Calculations 9543 1451 175 9543 1451 176 The Hauser-Feshbach statistical calculations were performed 9543 1451 177 with the COMNUC (Du70) and GNASH (Yo92b) codes. Both codes 9543 1451 178 include a double-humped fission barrier model, using uncoupled 9543 1451 179 oscillators for the barrier representation in GNASH and coupled 9543 1451 180 or uncoupled oscillators in COMNUC, as described by Arthur 9543 1451 181 (Ar82a). The COMNUC calculations include the possibility of 9543 1451 182 width-fluctuation corrections and corrections for class II 9543 1451 183 fluctuations (Ly74), which are needed at lower energies, whereas 9543 1451 184 GNASH provides the preequilibrium corrections that are required 9543 1451 185 at higher energies. Accordingly, COMNUC was used in the 9543 1451 186 calculations below about 2 MeV, utilizing a non-resonant model 9543 1451 187 and including class II fluctuations, and the GNASH code was 9543 1451 188 employed at higher energies using two uncoupled oscillators in 9543 1451 189 the fission calculations. 9543 1451 190 9543 1451 191 Each compound nucleus formed in the calculations is permitted 9543 1451 192 to decay through the fission channel, by neutron emission, and 9543 1451 193 by gamma-ray emission. Neutron transmission coefficients for 9543 1451 194 the Hauser-Feshbach calculations are obtained from the coupled- 9543 1451 195 channel optical model. Gamma ray transmission coefficients are 9543 1451 196 obtained from gamma-ray strength functions calculated with the 9543 1451 197 generalized Lorentzian model of Kopecky and Uhl (Ko90). 9543 1451 198 Transmission coefficients for fission are calculated from the 9543 1451 199 fission model summarized here and detailed in Yo92b. 9543 1451 200 9543 1451 201 Gilbert and Cameron (Gi70) phenomenological level density 9543 1451 202 functions were used to represent continuum levels at ground- 9543 1451 203 state deformations, appropriately matched to available 9543 1451 204 experimental structure data at lower excitation energies. 9543 1451 205 Multiplicative factors were applied to the level density 9543 1451 206 functions to account for enhancements in the fission transition 9543 1451 207 state densities at the fission barriers due to increased 9543 1451 208 asymmetry conditions, and the continuum level densities were 9543 1451 209 matched to the discrete fission transition states at each 9543 1451 210 barrier. The discrete fission transition state spectra were 9543 1451 211 calculated from bandhead information taken from calculations and 9543 1451 212 compilations by Britt (Br82) and by Nagel (Na91). 9543 1451 213 9543 1451 214 9543 1451 215 III. DESCRIPTION OF EVALUATED DATA BASE 9543 1451 216 9543 1451 217 A. Total Cross Section 9543 1451 218 9543 1451 219 The evaluated total cross section below 30 keV is obtained 9543 1451 220 from the resonance parameter evaluation in ENDF/B-VI, suitably 9543 1451 221 matched to the results of the current analysis at 30 keV. From 9543 1451 222 30 keV to 30 MeV, the coupled-channel deformed optical model 9543 1451 223 calculations described above were modified to agree with the 9543 1451 224 experimental data of Phillips (Ph70). 9543 1451 225 9543 1451 226 B. Elastic Cross Section 9543 1451 227 9543 1451 228 The elastic cross section at all energies is obtained from 9543 1451 229 the difference of the total and nonelastic cross sections. 9543 1451 230 Below 30 keV it comes from the ENDF/B-VI resonance parameters 9543 1451 231 and at higher energies it is mainly determined by the coupled- 9543 1451 232 channel optical model calculations. Angular distributions for 9543 1451 233 elastic neutrons were obtained at all energies from the coupled- 9543 1451 234 channel calculations and are given as Legendre expansions. 9543 1451 235 9543 1451 236 C. Fission Cross Section 9543 1451 237 9543 1451 238 The fission cross section was obtained by adjusting the 9543 1451 239 results of the theoretical analysis to optimize agreement with 9543 1451 240 experimental data. At most energies the adjustment was less 9543 1451 241 than a few percent. Above 8 MeV, the theoretical values were 9543 1451 242 used directly. Neutrons from fission are assumed to isotropic 9543 1451 243 in the laboratory system. 9543 1451 244 9543 1451 245 D. Radiative Capture Cross Section 9543 1451 246 9543 1451 247 The radiative capture cross section is calculated using the 9543 1451 248 generalized Lorentzian model of Ko90. The normalization of the 9543 1451 249 strength function was set by requiring the calculated (n,g) 9543 1451 250 cross section be consistent with measured values for 241Am. 9543 1451 251 9543 1451 252 E. Inelastic Neutron Cross Sections 9543 1451 253 9543 1451 254 Discrete (n,n') cross sections are included for the lowest 40 9543 1451 255 excited states of 241Am. The first, second, third, and fifth 9543 1451 256 excited states are members of the K = 5/2 ground-state 9543 1451 257 rotational band and include coupled-channel as well as compound 9543 1451 258 nucleus contributions. The remaining discrete-state cross 9543 1451 259 sections through the 40th excited state are combinations of 9543 1451 260 compound nucleus and preequilibrium contributions and were 9543 1451 261 calculated with the GNASH code. Angular distributions for all 9543 1451 262 the discrete inelastic neutrons are appropriate combinations of 9543 1451 263 the compound nucleus, direct reaction, and preequilibrium 9543 1451 264 contributions and are represented by Legendre expansions. 9543 1451 265 9543 1451 266 The inelastic data corresponding to excitation energies in 9543 1451 267 241Am above 0.508 MeV are given as energy-angle correlated 9543 1451 268 continuous spectra and were calculated with the GNASH code. The 9543 1451 269 results are given in File 6 of the ENDF/B-formatted evaluation 9543 1451 270 (ENDF-6 format) and utilize systematics by Kalbach (Ka88) for 9543 1451 271 angular distribution information, parameterized in terms of 9543 1451 272 preequilibrium ratios calculated in GNASH. 9543 1451 273 9543 1451 274 F. Cross Sections for 241Am(n,xn) Reactions 9543 1451 275 9543 1451 276 The 241Am(n,2n), (n,3n), and (n,4n) cross sections result 9543 1451 277 entirely from the theoretical analysis and GNASH calculations. 9543 1451 278 Energy-angle correlated distributions are given for all the 9543 1451 279 241Am(n,xn) reactions, making use of Kalbach's systematics 9543 1451 280 (Ka88) and the ENDF-6 File 6 representation. 9543 1451 281 9543 1451 282 G. Nubar 9543 1451 283 9543 1451 284 The evaluation of delayed nubar was carried over directly 9543 1451 285 from the ENDF/B-VI evaluation of 241Am. The prompt nubar 9543 1451 286 evaluation was obtained using Madland-Nix theory. 9543 1451 287 9543 1451 288 H. Fission Neutron Spectra 9543 1451 289 9543 1451 290 The fission neutron spectra was determined using Madland-Nix 9543 1451 291 theory and are consistent with nubar. 9543 1451 292 9543 1451 293 9543 1451 294 **************************************************************** 9543 1451 295 9543 1451 296 REFERENCES 9543 1451 297 9543 1451 298 Ar82 E. D. Arthur, "Use of the Statistical Model for the 9543 1451 299 Calculation of Compound Nucleus Contributions to Inelastic 9543 1451 300 Scattering on Actinide Nuclei," Proc. of OECD/NEA Specialists' 9543 1451 301 Meeting on Fast Neutron Scattering on Actinide Nuclei, (Paris, 9543 1451 302 November, 1981), NEANDC-158 "U" (1982) p. 145. 9543 1451 303 9543 1451 304 Ba74 B. B. Back, O. Hansen, H. C. Britt, and J. D. Garrett, 9543 1451 305 "Fission of Doubly Even Actinide Nuclei Induced by Direct 9543 1451 306 Reactions, " Phys. Rev. C 9, 1924 (1974). 9543 1451 307 9543 1451 308 Br82 H. C. Britt, personal communication, 1982. 9543 1451 309 9543 1451 310 Du70 C. L. Dunford, "A Unified Model for Analysis of Compound 9543 1451 311 Nucleus Reactions,"AI-AEC-12931, Atomics Int. (1970). 9543 1451 312 9543 1451 313 Gi65 A. Gilbert and A. G. W. Cameron, "A Composite Nuclear- 9543 1451 314 Level Density Formula with Shell Corrections," Can. J. Phys. 43, 9543 1451 315 1446 (1965). 9543 1451 316 9543 1451 317 Ka88 C. Kalbach, "Systematics of Continuum Angular 9543 1451 318 Distributions: Extensions to Higher Energies," Phys. Rev. C37, 9543 1451 319 2350 (1988); C. Kalbach and F. M. Mann, "Phenomenology of 9543 1451 320 Continuum Angular Distributions. I. Systematics and 9543 1451 321 Parameterization," Phys. Rev. C 23, 112 (1981). 9543 1451 322 9543 1451 323 Ko90 J. Kopecky and M.Uhl, "Test of Gamma-Ray Strength 9543 1451 324 Functions in Nuclear Reaction Model Calculations," Phys. Rev. C 9543 1451 325 42, 1941 (1990). 9543 1451 326 9543 1451 327 Ra70 J. Raynal, "Optical-Model and Coupled-Channel Calculations 9543 1451 328 in Nuclear Physics," IAEA SMR-9/8, Int. At. En. Agency (1970). 9543 1451 329 9543 1451 330 Yo88 P. G. Young and E. D. Arthur, "Calculation of 235U(n,n') 9543 1451 331 Cross Sections for ENDF/B-VI," Int. Conf. on Nucl. Data for 9543 1451 332 Science and Technology, Mito, Japan, May 30 - June 3, 1988 (Ed. 9543 1451 333 S. Igarasi, Saikon Publ. Co., Ltd., 1988) p. 603. 9543 1451 334 9543 1451 335 Yo92a P. G. Young and E. D. Arthur, "Theoretical Analyses of 9543 1451 336 (n,xn) Reactions on 235U, 238U, 237Np, and 239Pu for ENDF/B-VI," 9543 1451 337 Proc. Int. Conf. on Nuclear Data for Science and Technology, 9543 1451 338 Julich, Germany, 13-17 May 1991 (LA-UR-91-1424), [Ed. S. M. 9543 1451 339 Qaim, Springer-Verlag, Germany (1992)], p. 894. 9543 1451 340 9543 1451 341 Yo92b P. G. Young, E. D. Arthur, and M. B. Chadwick, 9543 1451 342 "Comprehensive Nuclear Model Calculations: Introduction to the 9543 1451 343 Theory and Use of the GNASH Code," Los Alamos National 9543 1451 344 Laboratory report LA-12343-MS (1992). 9543 1451 345 9543 1451 346 **************************************************************** 9543 1451 347 *****************************************************************9543 1451 348 9543 1451 349 THE COMMENTS BELOW PERTAIN TO THE PARTS OF THE ENDF/B-VI 9543 1451 350 EVALUATION THAT ARE UTILIZED HERE. 9543 1451 351 9543 1451 352 *****************************************************************9543 1451 353 REVISION 1 CHANGES 9543 1451 354 ENERGY RELEASE PER FISSION FROM ENDF/B-V ADDED 9543 1451 355 9543 1451 356 * * * * * * *9543 1451 357 HISTORY 9543 1451 358 THE ORIGINAL EVALUATION WAS PERFORMED BY 9543 1451 359 GU FUHUA, YU BAOSHENG, ZHOU DELIN, ZHUANG YOUXIANG 9543 1451 360 SHI XIANGJUN, YAN SHIWEI, WANG CUILAN, ZHANG JENGSHANG 9543 1451 361 UNDER THE CONTRACTS BETWEEN IAEA/NDS AND IAE,1985. 1| AND 9543 1451 362 REVISED BY 9543 1451 363 ZHOU DELIN, YU BAOSHENG, LIU TONG 9543 1451 364 SHI XIANGJUN, YAN SHIWEI 9543 1451 365 1988. 2| THE CAPTURE CROSS SECTIONS AND RESONANCE PARAMETERS 9543 1451 366 HAVE BEEN REVIEWED AND REEVALUATED BY ZHOU DELIN ET AL.1988 3|.9543 1451 367 MF=1, GENERAL INFORMATION 9543 1451 368 MT=451, COMMENTS AND DICTIONARY 9543 1451 369 MT=452, TOTAL NUMBER OF NEUTRONS PER FISSION 9543 1451 370 IT IS THE SUM OF DELAY NEUTRONS (MT=455) AND PROMPT 9543 1451 371 NEUTRONS PER FISSION (MT=456). 9543 1451 372 MT=455, T.R.ENGLAND +,LA-11151,LA-11534,LAURA-88-4118 9543 1451 373 MF=2, MT=151, RESONANCE PARAMETERS 9543 1451 374 RESOLVED RESONANCE PARAMETERS FOR SLBW FORMULA IN 1.0E-5 TO 9543 1451 375 1.5E+2 EV RESONANCE ENERGY REGION 9543 1451 376 RESOLVED PARAMETERS WERE RECOMMENDED AS FOLLOWING: 9543 1451 377 IT WAS NOTICED THAT THE PARAMETERS OF THE FIRST SEVERAL WELL 9543 1451 378 DEFINED RESONANCES (0.308, 0,576, 1.276, 1.928, 2.372, 2.358 9543 1451 379 EV, FOR EXAMPLE) GIVEN BY DERRIEN ET AL. 5| (TRANSMISSION), 9543 1451 380 KALEBIN ET AL. 6| (TRANSMISSION) AS WELL AS WESTON ET AL. 7| 9543 1451 381 (ABSORPTION, NOMALIZED TO THERMAL CAPTURE CROSS SECTION OF 582 9543 1451 382 B) RESPECTIVELY ARE IN EXCELLENT AGREEMENT WITH EACH OTHER. 9543 1451 383 THIS FACT MEANS THAT THE RESONANCE PARAMETERS FOR THE FULL 9543 1451 384 RESONANCE ENERGY REGION CAN BE COMBINED BY AVERAGING WEIGHTED 9543 1451 385 WITH RANDOM ERROR ONLY WITHOUT TAKING THE 8% SYSTEMATIC ERROR 9543 1451 386 IN ABSORPTION MEASUREMENT 7| INTO ACCOUNT. SO THAT THE 9543 1451 387 RECOMMENDED VALUES FOR MOST RESONANCES WERE AVERAGED IN EQUAL 9543 1451 388 WEIGHT EXCEPT THOSE FOR WHICH THE RANDOM ERRORS OF WESTON ET 9543 1451 389 AL.'S MEASUREMENT OR/AND THE ERRORS OF KALEBIN ET AL.'S 9543 1451 390 MEASUREMENT ARE MUCH LARGER THAN DERRIEN ET AL.'S, IN SUCH 9543 1451 391 CASES THE AVERAGE WERE MADE WITH UNEQUAL WEIGHTS PROPERLY. 9543 1451 392 UNRESOLVED RESONANCE PARAMETERS IN 1.5E+2 EV TO 30 KEV ENERGY 9543 1451 393 REGION 9543 1451 394 KIKUCH'S PARAMETERS 4| WERE USED AS INPUT DATA AND ADJUSTED 9543 1451 395 TO FIT THE CAPTURE CROSS SECTIONS (EVALUATED ON THE BASES OF 9543 1451 396 WESTON ET AL.'S, VANPRAET ET AL.'S 8|, WISSHAK ET AL.'S 9| 9543 1451 397 AND DERRIEN ET AL.'S MEASUREMENTS) AND FISSION CROSS SECTION 9543 1451 398 OF DABBS 10| (AVERAGED IN PROPER ENERGY RANGE) THEN THE 9543 1451 399 RECOMMENDED UNRESOLVED RESONANCE PARAMETERS WERE OBTAINED. 9543 1451 400 THERMAL ENERGY CROSS SECTIONS 9543 1451 401 FISSION CROSS SECTION THE VALUE OF 3.15 B WAS ADOPTED. 9543 1451 402 CAPTURE CROSS SECTION 620+-13 B, THE WEIGHTED AVERAGED VALUE 9543 1451 403 OF THE FOLLOWING DATA WAS ADOPTED: 9543 1451 404 .KALEBIN: 625+-20 (=640-3.15-11.5, TRANSMISSION); 9543 1451 405 .DOVBENKO ET AL.: 654+-104 (CAPTURE) 11|; 9543 1451 406 .HARBOUR ET AL.: 612+-25 (CAPTURE, DEDUCED RESULT TAKEN FROM 9543 1451 407 AN ANALYSIS BY STORY, 1978. QUOTTED FROM LYNN ET AL.) 12|; 9543 1451 408 .POMERANCE: 625+-35 (QUOTED FROM LYNN ET AL.) 12|; 9543 1451 409 .WISSHAK ET AL.: 625+-35 (ISOMERIC RATIO, INDIRECTLY) 13|; 9543 1451 410 .WESTON ET AL.: 582+-50 (ABSORPTION, A RELATIVE MEASUREMENT 9543 1451 411 NORMALIZED TO THERMAL CAPTURE CROSS SECTION OF 582 B. IT MAY 9543 1451 412 BE CONSIDERED TO NORMALIZE TO DERRIEN'S MEASUREMENT AT FIRST 9543 1451 413 SEVERAL RESONANCES EQUIVALENTLY. THEN THE 8% SYSTEMATIC 9543 1451 414 UNCERTAINTY IN THE ENERGY REGION OF >0.2 EV MUST BE ADDED TO 9543 1451 415 THERMAL VALUE) 3|. 9543 1451 416 MF=4 ANGULAR DISTRIBUTIONS OF SECONDARY NEUTRONS 9543 1451 417 MT=18 ANGULAR DISTRIBUTIONS OF FISSION NEUTRONS 9543 1451 418 ASSUMED ISOTROPIC IN THE LABORATORY SYSTEM. 9543 1451 419 MF=9 9543 1451 420 MT=102 9543 1451 421 THE DATA OF ISOMERIC RATIO HAVE BEEN REVISED BASED ON THE NEW 9543 1451 422 EVALUATION 2! AND THE SHAPE OF THE THEORETICAL CALCULATION OF 9543 1451 423 13! . 9543 1451 424 MF=12,13,14,15 9543 1451 425 THE DATA CALCULATED BY R. HOWERTON (P.C.) FROM MF=2,3,5. 9543 1451 426 MF=32,33 9543 1451 427 THE FILE 32 AND 33 OF ENDF/B-V, REV.2 ARE ADOPTED. BUT THE 9543 1451 428 THE COVARIANCES OF MT=151 OF FILE 32 AND THE COVARIANCES OF 9543 1451 429 MT=18 OF FILE 33 HAVE BEEN MODIFIED PRELIMINARYLY TO MATCH 9543 1451 430 THE PRESENT EVALUATIONS. 9543 1451 431 9543 1451 432 REFERENCES 9543 1451 433 1| GU FUHUA ET AL., NEUTRON DATA EVALUATION FOR AM-241, 9543 1451 434 1985.(UNPUBLISHED). 9543 1451 435 2| THOU DELIN ET AL., NEUTRON DATA EVALUATION FOR AM-241, 9543 1451 436 1988. (UNPUBLISHED). 9543 1451 437 3| ZHOU DELIN , ON THE CAPTURE DATA EVALUATION FOR 9543 1451 438 AM-241, 1988. (TO BE PUBLISHED). 9543 1451 439 4| KIKUCH Y., JAERI-M 82-096, 1982. 9543 1451 440 5| DERRIEN H. ET AL., WASH75 P.637, 1975. 9543 1451 441 6| KALEBIN S. ET AL., A.E. 40, 373 (1976). 9543 1451 442 7| WESTON L. ET AL., NUCL. SCI. ENG., 61, 356 (1976). 9543 1451 443 8| VANPRAET . ET AL., SANTA FE(85), P.493, 1985. 9543 1451 444 9| WISSHAK K. ET AL., NUCL. SCI. ENG., 76, 148 (1980). 9543 1451 445 10| DABBS J. ET AL., NUCL. SCI. ENG., 83, 22 (1983). 9543 1451 446 11| DOVBENKO A. ET AL., LA-TR-71-74, 1971. 9543 1451 447 12| LYNN J. ET AL., PROGRESS IN NUCLEAR ENERGY, V.5, 9543 1451 448 P.255, 1980. 9543 1451 449 HARBOUR R. ET AL., NUCL. SCI. ENG., 50, 364 (1973). 9543 1451 450 POMERANCE H. ORNL-1879, P.50, 1955. 9543 1451 451 13| WISSHAK K. ET AL., NUCL. SCI. ENG., 81, 396 (1982). 9543 1451 452 **************************************************************** 9543 1451 453 1 451 579 39543 1451 454 1 452 37 49543 1451 455 1 455 7 49543 1451 456 1 456 37 49543 1451 457 1 458 5 49543 1451 458 2 151 419 49543 1451 459 3 1 124 49543 1451 460 3 2 124 49543 1451 461 3 4 40 49543 1451 462 3 16 13 49543 1451 463 3 17 10 49543 1451 464 3 18 87 49543 1451 465 3 37 11 49543 1451 466 3 51 40 49543 1451 467 3 52 39 49543 1451 468 3 53 38 49543 1451 469 3 54 37 49543 1451 470 3 55 37 49543 1451 471 3 56 37 49543 1451 472 3 57 36 49543 1451 473 3 58 35 49543 1451 474 3 59 35 49543 1451 475 3 60 34 49543 1451 476 3 61 34 49543 1451 477 3 62 33 49543 1451 478 3 63 33 49543 1451 479 3 64 32 49543 1451 480 3 65 32 49543 1451 481 3 66 31 49543 1451 482 3 67 31 49543 1451 483 3 68 30 49543 1451 484 3 69 30 49543 1451 485 3 70 29 49543 1451 486 3 71 29 49543 1451 487 3 72 28 49543 1451 488 3 73 28 49543 1451 489 3 74 28 49543 1451 490 3 75 27 49543 1451 491 3 76 27 49543 1451 492 3 77 27 49543 1451 493 3 78 26 49543 1451 494 3 79 26 49543 1451 495 3 80 25 49543 1451 496 3 81 25 49543 1451 497 3 82 25 49543 1451 498 3 83 24 49543 1451 499 3 84 24 49543 1451 500 3 85 23 49543 1451 501 3 86 23 49543 1451 502 3 87 23 49543 1451 503 3 88 22 49543 1451 504 3 89 22 49543 1451 505 3 90 22 49543 1451 506 3 91 22 49543 1451 507 3 102 30 49543 1451 508 4 2 107 49543 1451 509 4 18 2 49543 1451 510 4 51 105 49543 1451 511 4 52 103 49543 1451 512 4 53 101 49543 1451 513 4 54 52 49543 1451 514 4 55 101 49543 1451 515 4 56 52 49543 1451 516 4 57 52 49543 1451 517 4 58 52 49543 1451 518 4 59 52 49543 1451 519 4 60 52 49543 1451 520 4 61 50 49543 1451 521 4 62 50 49543 1451 522 4 63 50 49543 1451 523 4 64 50 49543 1451 524 4 65 50 49543 1451 525 4 66 50 49543 1451 526 4 67 50 49543 1451 527 4 68 50 49543 1451 528 4 69 48 49543 1451 529 4 70 48 49543 1451 530 4 71 48 49543 1451 531 4 72 48 49543 1451 532 4 73 48 49543 1451 533 4 74 48 49543 1451 534 4 75 48 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